Nonreciprocity reversal of magnetoacoustic attenuation in NiFe alloy thin films

Abstract

Nonreciprocity, the asymmetry of transport, underlies technologies from the diode to the microwave isolator. In a ferromagnet, a surface acoustic wave generates an elliptical effective field with propagation-locked handedness, breaking the reciprocity of its propagation. Despite decades of study on this phenomenon, a method for controlling the sign of the nonreciprocity has remained elusive. Here we observe a sign reversal in Ni$_x$Fe$_{100-x}$ films. A 0.8 at.% change across Permalloy's zero-magnetostriction composition, where the magnetoelastic coefficient $b$ changes sign, reverses the handedness of the elliptical effective field and thereby the nonreciprocity, from 78.6% to -61.8%. Angle-dependent measurements and spin-wave-ellipticity modelling show that reversing the sign of $b$ reverses the handedness of the elliptically polarized effective field. Aided by cubic frequency scaling, we resolve the sign of $b$ down to -0.05 MPa in a 10-nm film, establishing nonreciprocity as a nanoscale probe of magnetoelastic coupling.