Non-monotonic dependence of OAM Schmidt spectrum on crystal thickness

Abstract

The orbital angular momentum (OAM) of photons provides a high-dimensional resource for quantum information protocols. The dimensionality of OAM-entangled states generated via spontaneous parametric down-conversion (SPDC) is quantified by the angular Schmidt spectrum. Here, we experimentally investigate the dependence of the angular Schmidt spectrum on the thickness of the nonlinear crystal. Contrary to previous studies reporting a monotonic decrease in the Schmidt number with increasing crystal thickness, we report the first experimental observation of a nonmonotonic behavior, as we demonstrate an increase in the Schmidt number beyond a certain crystal thickness. We attribute this to the spatial walk-off effect in the anisotropic nonlinear crystal and explain it using a theoretical model that is devoid of standard phase-matching approximations. These findings can have important implications for high-dimensional entangled state generation.