Topologically Configurable Nonlinear Vortex Generation at van der Waals Heterostructures

Abstract

van der Waals (vdW) materials offer a highly tunable and efficient platform at nanoscale for nonlinear and quantum optics. Twist-stacked vdW heterostructures enable elegant control of symmetry and interlayer coupling. Prior studies mainly focus on planar twisted interfaces, while neglecting the naturally formed and mandatory defects in such vdW heterostructures. Here, we demonstrate nonlinear singular optics with topologically configurable nonlinear vortex generation at the corner singularity of vdW heterostructures. By tailoring azimuthally discrete second-harmonic phase gradients at each interface, we obtain programmable nonlinear vortex emitters with dominant target OAM components. Nonlinear OAM beams with topological charge $\ell = 1$ and $\ell = -2$ are experimentally realized, respectively. Our work unlocks the untapped potentials of nonlinear singular optics in twisted vdW materials as a reconfigurable and lithography-free platform for nonlinear structured light generation, important in quantum nonlinear optics and related fields.