Universal thermal breakdown of polaron coherence in one, two, and three dimensions

Abstract

How a polaron loses its quasiparticle coherence with increasing temperature is a long-standing open problem. Holstein addressed it in 1959 only in the extreme antiadiabatic, strong-coupling limit, while more recent numerically exact approaches are largely restricted to one dimension. Here we solve this problem on square and simple cubic lattices across the weak-, intermediate-, and strong-coupling regimes. We show that the polaron effective mass $m^*$ and inverse lifetime $1/τ$ increase monotonically with temperature until, at $T \sim 0.5\,Ω$, the quasiparticle peak dissolves into a broad incoherent thermal continuum. The phonon frequency $Ω$ therefore defines a universal coherence scale, independent of dimensionality and coupling strength, validating Holstein's prediction far beyond the regime in which it was derived. These results follow from a finite-temperature generalization of the Momentum Average (MA) approximation, yielding a closed-form, diagrammatically derived self-energy that is asymptotically exact in the strong-coupling limit at all temperatures. Benchmark comparisons demonstrate excellent quantitative agreement of the resulting 1D spectral functions with the numerically exact Variational Exact Diagonalization-Finite-Temperature Lanczos Method (VED-FTLM) and finite-$T$ Density Matrix Renormalization Group (DMRG).