Influence of twist direction and large deformation on soft material torsional contact

Abstract

Shear-induced contact area reduction is widely observed in soft contacts, yet recent torsional experiments have revealed a more complex non-monotonic evolution in which the contact area first increases and then decreases with twist angle. The mechanism responsible for this initial area increase and the role of large deformation in the overall area evolution remain unclear. In this study, we experimentally investigate the torsional contact response of soft Polydimethylsiloxane (PDMS) spheres by combining forward-backward twist tests with a systematic variation of the curing-agent-to-base ratio to tune material softness and deformation level. The loading-unloading tests show that the torsional interface is strongly irreversible: during unloading, the contact area follows a decrease-increase-decrease path rather than retracing the loading branch, and repeatable petal-like edges appear, indicating a wrinkle-induced surface instability. By decreasing the mixing ratio, we find that larger deformation strengthens the area-reduction contribution and eventually suppresses the initial area increase, leading to a monotonic area decrease during loading for sufficiently soft PDMS. Softer PDMS also exhibits lower shear strength, weaker torque oscillations, and improved repeatability. The results provide experimental evidence that large deformation can drive shear-induced contact area reduction, while the origin of the initial area increase remains unresolved. These findings narrow the possible mechanisms (e.g., triboelectrification) responsible for the initial area increase and provide a stringent benchmark for frictional contact models of soft interfaces.