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Predictive wavelength tailoring of uniform GaSb-based quantum dots for emission at 1.55 um

Markus Peil, Maja Wasiluk, Ziemowit Olinkiewicz, Tymon Przychodni, Robert Matysiak, Teemu Taskinen, Joona Salonen, Abhiroop Chellu, Metin Patli, Joonas Hilska, Anna Musiał, Michał Gawełczyk, Mircea Guina, Teemu Hakkarainen

cond-mat.mes-hallarXiv:2608.30628

Abstract

A detailed study of emission wavelength tailoring of GaSb-based QDs formed by InGaSb-filling of droplet-etched nanoholes in AlGaSb is presented. The study shows that the emission wavelength can be modified from 1.48 um to the center of the telecom C-band at 1.55 mm by independently varying the QD composition and size. More specifically, the optical transition energy shifts linearly as a function of In-content of the QD material at a rate of -4.4 meV/In-percentage, and with the number of monolayers (ML) of material used for filling the nanoholes, at -2.0 meV/ML. These experimentally observed energy shifts are well predicted by simulations yielding rates of -4.3 meV/In-percentage and -2.1 meV/ML, respectively. For the simulation, a uniform In composition, low intermixing, and microscopically measured QD geometry is considered. Additionally, excellent ensemble QD uniformity, with unprecedented inhomogeneous broadening well-below 7 meV across all samples is demonstrated. Finally, photoluminescence of single-QDs reveals narrow excitonic emission lines of 13.8+/-6.7 ueV and low fine-structure splitting values reaching <10 ueV. These results identify GaSb-based LDE QDs as a tunable telecom platform for scaling quantum-photonic applications over long-haul optical fiber networks.

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