Coherent antiferromagnetic resonance in MnO driven by impulsive terahertz excitation

Abstract

Antiferromagnets (AFMs) offer a promising platform for ultrafast information processing owing to their intrinsically fast spin dynamics and vanishing net magnetization. Realizing this potential, however, requires understanding how terahertz fields excite coherent magnons and how the resulting spin motion is transduced into an optical signal. Here we report impulsive terahertz (THz) excitation and time-domain detection of the antiferromagnetic resonance (AFMR) in single-crystal manganese(II) oxide. Time-resolved birefringence measurements reveal long-lived coherent spin oscillations in the AFM phase. The resonance softens and becomes strongly damped upon warming toward the Néel temperature. Despite this similar excitation behavior, the detected birefringence in MnO is markedly weaker than in NiO. We associate this suppressed optical visibility with the weak spin--orbit-mediated magneto-optical coupling of orbital-singlet, high-spin Mn$^{2+}$. These results demonstrate that coherent magnon excitation and its optical detection are governed by distinct microscopic interactions.