Room-temperature Magnetoelastic Coupling in UIr$_4$Al$_{15}$

Abstract

The interplay between electronic and structural degrees of freedom underpins many emergent phenomena in quantum materials, yet magnetoelastic coupling in metallic systems is typically weak and confined to low temperatures or microscopic length scales. Here, we report giant magnetoelastic coupling slightly above room temperature in the uranium-based intermetallic compound UIr$_4$Al$_{15}$. Using temperature-dependent single-crystal X-ray diffraction together with anisotropic magnetic susceptibility measurements, we directly resolve subtle but reproducible structural distortions coupled to magnetic alignment. Despite the absence of crystallographic symmetry breaking, pronounced anomalies emerge in lattice parameters and selected chemical bond distances near the magnetic transition region, revealing an unusual sensitivity of the crystal structure to magnetic orientation. The coupling enables direct probing of how atomic distances and local chemical bonding govern the electronic and magnetic states in a bulk intermetallic material. Our results establish UIr$_4$Al$_{15}$ as a rare platform in which magnetism and lattice distortions are strongly intertwined near room temperature, opening new opportunities for magnetically responsive quantum materials and functional magnetic sensing applications.