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Abrupt Transition between Thermally-Activated Relaxation and Quantum Tunneling in a Molecular Magnet

K. M. Mertes, Y. Zhong, M. P. Sarachik, Y. Paltiel, H. Shtrikman, E. Zeldov, E. Rumberger, D. N. Hendrickson

cond-mat.mes-hallarXiv:cond-mat/0012247

Abstract

We report Hall sensor measurements of the magnetic relaxation of Mn12 acetate as a function of magnetic field applied along the easy axis of magnetization. Data taken at a series of closely-spaced temperatures between 0.24 K and 1.4 K provide strong new evidence for an abrupt ``first-order'' transition between thermally-assisted relaxation and magnetic decay via quantum tunneling.

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