Abrupt Transition between Thermally-Activated Relaxation and Quantum Tunneling in a Molecular Magnet

Abstract

We report Hall sensor measurements of the magnetic relaxation of Mn12 acetate as a function of magnetic field applied along the easy axis of magnetization. Data taken at a series of closely-spaced temperatures between 0.24 K and 1.4 K provide strong new evidence for an abrupt ``first-order'' transition between thermally-assisted relaxation and magnetic decay via quantum tunneling.

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