Particle tunneling through a polarizable insulator

Abstract

The tunneling probability between two leads connected by a molecule, a chain, a film, or a bulk polarizable insulator is investigated within a model of an electron tunneling from lead A to a state higher in energy, describing the barrier, and from there to lead B. To describe the possibility of energy exchange with excitations of the molecule or the insulator we couple the intermediate state to a single oscillator or to a spectrum of these, respectively. In the single-oscillator case we find for weak coupling that the tunneling is weakly suppressed by a Debye-Waller-type factor. For stronger coupling the oscillator gets 'stiff' and we observe a suppression of tunneling since the effective barrier is increased. The probability for the electron to excite the oscillator increases with the coupling. In the case of a film, or a bulk barrier the behavior is qualitatively the same as in the single oscillator case. An insulating chain, as opposed to a film or a bulk connecting the two leads,shows an 'orthogonality catastrophe' similar to that of an electronic transition in a Fermi gas.