Experimental study of MnCl3(C12H8N2) - an S = 2 Heisenberg antiferromagnetic chain
E. Cizmar, J. -H. Park, S. J. Gamble, B. H. Ward, D. R. Talham, J. van Tol, L. -C. Brunel, M. Orendac, A. Feher, J. Sebek, M. W. Meisel
Abstract
The thermodynamic and magnetic properties of MnCl3(C12H8N2), have been studied down to 2 K. The material is an S = 2 antiferromagnetic linear chain that undergoes long-range ordering to a canted antiferromagnetic state at 23 K. The comparison of magnetic data from polycrystalline samples with the results of specific heat measurements using a pressed pellet of powder reveals the importance of the length of the chains in the sample in relation to the magnetic correlation length.
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