Magnetism in Atomic-Sized Palladium Contacts and Nanowires
Abstract
We have investigated Pd nanowires theoretically, and found that, unlike either metallic or free atomic Pd, they exhibit Hund's rule magnetism. In long, monoatomic wires, we find a spin moment of 0.7 Bohr magnetons per atom, whereas for short, monoatomic wires between bulk leads, the predicted moment is about 0.3 Bohr magnetons per wire atom. In contrast, a coaxial (6,1) wire was found to be nonmagnetic. The origin of the wire magnetism is analyzed.
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