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Time-Reversal Symmetry-Breaking Superconductivity in Heavy Fermion PrOs4Sb12 detected by Muon Spin Relaxation

Y. Aoki, A. Tsuchiya, T. Kanayama, S. R. Saha, H. Sugawara, H. Sato, W. Higemoto, A. Koda, K. Ohishi, K. Nishiyama, R. Kadono

cond-mat.supr-conarXiv:cond-mat/0308196

Abstract

We report on muon spin relaxation measurements of the 4f2-based heavy-fermion superconductor filled-skutterudite PrOs4Sb12. The results reveal the spontaneous appearance of static internal magnetic fields below the superconducting transition temperature, providing unambiguous evidence for the breaking of time-reversal symmetry in the superconducting state. A discussion is made on which of the spin or orbital component of Cooper pairs carries a nonzero momentum.

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