Series of Bulk Magnetic Phase Transitions in NaxCoO2: a muSR study
P. Mendels, D. Bono, J. Bobroff, G. Collin, D. Colson, N. Blanchard, H. Alloul, I. Mukhamedshin, F. Bert, A. Amato, A. D. Hillier
Abstract
Using muon spin rotation, well-defined bulk ~ 100% magnetic phases in NaxCoO2 are revealed. A novel magnetic phase is detected for x = 0.85 with the highest transition temperature ever observed for x >= 0.75. This stresses the diversity of x >=0.75 magnetic phases and the link between magnetic and structural degrees of freedom. For the charge-ordered x = 0.50 compound, a cascade of transitions is observed below 85 K. From a detailed analysis of our data, we conclude that the ordered moment varies continuously with temperature and suggest that the two secondary transitions at 48 K and 29 K correspond to a moderate reorientation of antiferromagnetically coupled moments.
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