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Decoupling of self-diffusion and structural relaxation during a fragile-to-strong crossover in a kinetically constrained lattice gas

Albert C. Pan, Juan P. Garrahan, David Chandler

cond-mat.stat-mecharXiv:cond-mat/0501739

Abstract

We present an interpolated kinetically constrained lattice gas model which exhibits a transition from fragile to strong supercooled liquid behavior. We find non-monotonic decoupling that is due to this crossover and is seen in experiment.

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