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Magnetic Order and Spin Dynamics in Ferroelectric HoMnO3

O. P. Vajk, M. Kenzelmann, J. W. Lynn, S. B. Kim, S. -W. Cheong

cond-mat.str-elarXiv:cond-mat/0502006

Abstract

Hexagonal HoMnO3 is a frustrated antiferromagnet (TN=72 K) ferroelectric (TC=875 K) in which these two order parameters are coupled. Our neutron measurements of the spin wave dispersion for the S=2 Mn3+ on the layered triangular lattice are well described by a two-dimensional nearest-neighbor Heisenberg exchange J=2.44 meV, and an anisotropy D that is 0.093 meV above the spin reorientation transition at 40 K, and 0.126 meV below. For H c the magnetic structures and phase diagram have been determined, and reveal additional transitions below 8 K where the ferroelectrically displaced Ho3+ ions are ordered magnetically.

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