Tunable Resonant Raman Scattering from Singly Resonant Single Wall Carbon Nanotubes
Y. Yin, A. G. Walsh, A. N. Vamivakas, S. Cronin, A. M. Stolyarov, M. Tinkham, W. Bacsa, M. S. Unlu, B. B. Goldberg, A. K. Swan
Abstract
We perform tunable resonant Raman scattering on 17 semiconducting and 7 metallic singly resonant single wall carbon nanotubes. The measured scattering cross-section as a function laser energy provides information about a tube's electronic structure, the lifetime of intermediate states involved in the scattering process and also energies of zone center optical phonons. Recording the scattered Raman signal as a function of tube location in the microscope focal plane allows us to construct two-dimensional spatial maps of singly resonant tubes. We also describe a spectral nanoscale artifact we have coined the "nano-slit effect".
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