Critical spin liquid at 1/3 magnetization in a spin-1/2 triangular antiferromagnet

Abstract

Although magnetically ordered at low temperatures, the spin-1/2 triangular antiferromagnet Cs2CuCl4 exhibits remarkable spin dynamics that strongly suggest proximity to a spin liquid phase. Here we address the question of whether a proximate spin liquid may also occur in an applied magnetic field, leaving a similar imprint on the dynamical spin correlations of this material. Specifically, we explore a spatially anisotropic Heisenberg spin-1/2 triangular antiferromagnet at 1/3 magnetization from a dual vortex perspective, and indeed find a new ``critical'' spin liquid phase described by QED3 with an emergent SU(6) symmetry. A number of nontrivial predictions are given for the dynamical spin structure factor in this ``algebraic vortex liquid'' phase, which can be tested experimentally via inelastic neutron scattering. We also discuss how the well-studied ``up-up-down'' magnetization plateaus can be captured within our approach, and further predict the existence of a stable gapless solid phase in a weakly ordered up-up-down state. Finally, we predict several anomalous ``roton'' minima in the excitation spectrum in the regime of lattice anisotropy where the canted Neel state appears.

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