Elastic Spin Relaxation Processes in Semiconductor Quantum Dots

Abstract

Electron spin decoherence caused by elastic spin-phonon processes is investigated comprehensively in a zero-dimensional environment. Specifically, a theoretical treatment is developed for the processes associated with the fluctuations in the phonon potential as well as in the electron procession frequency through the spin-orbit and hyperfine interactions in the semiconductor quantum dots. The analysis identifies the conditions (magnetic field, temperature, etc.) in which the elastic spin-phonon processes can dominate over the inelastic counterparts with the electron spin-flip transitions. Particularly, the calculation results illustrate the potential significance of an elastic decoherence mechanism originating from the intervalley transitions in semiconductor quantum dots with multiple equivalent energy minima (e.g., the X valleys in SiGe). The role of lattice anharmonicity and phonon decay in spin relaxation is also examined along with that of the local effective field fluctuations caused by the stochastic electronic transitions between the orbital states. Numerical estimations are provided for typical GaAs and Si-based quantum dots.