Spin Gaps and Bilayer Coupling in YBa2Cu3O7-δ and YBa2Cu4O8

Abstract

We investigate the relevance to the physics of underdoped YBa2Cu3O 6+x and YBa2Cu4O8 of the quantum critical point which occurs in a model of two antiferromagnetically coupled planes of antiferromagnetically correlated spins. We use a Schwinger boson mean field theory and a scaling analysis to obtain the phase diagram of the model and the temperature and frequency dependence of various susceptibilities and relaxation rates. We distinguish between a low ω ,T coupled-planes regime in which the optic spin excitations are frozen out and a high ω ,T decoupled-planes regime in which the two planes fluctuate independently. In the coupled-planes regime the yttrium nuclear relaxation rate at low temperatures is larger relative to the copper and oxygen rates than would be naively expected in a model of uncorrelated planes. Available data suggest that in YBa2Cu4O8 the crossover from the coupled to the decoupled planes regime occurs at T 700K or T 200K. The predicted correlation length is of order 6 lattice constants at T=200K. Experimental data related to the antiferromagnetic susceptibility of YBa2Cu4O8 may be made consistent with the theory, but available data for the uniform susceptibility are inconsistent with the theory.

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