Two--magnon scattering and the spin--phonon interaction beyond the adiabatic approximation

Abstract

We consider a model of Raman scattering for a two--dimensional S=1/2 Heisenberg Anti-Ferromagnet which includes a dynamical spin--phonon interaction. We observe a broadening of the line shape due to increased coupling with excited high--energy spin states. Our results are close to a model of random static exchange interactions, first introduced in this context by Haas et al. [J. Appl. Phys. 75, 6340, (1994)], which, when extended to large numbers of spins, explains experiments in the parent insulating compounds of high-Tc superconductors.

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