Temperature-dependent spin gap and singlet ground state in BaCuSi2O6
Y. Sasago, K. Uchinokura, A. Zheludev, G. Shirane
Abstract
Bulk magnetic measurements and inelastic neutron scattering were used to investigate the spin-singlet ground state and magnetic gap excitations in BaCuSi2O6, a quasi-2-dimensional antiferromagnet with a bilayer structure. The results are well described by a model based on weakly interacting antiferromagnetic dimers. A strongly temperature-dependent dispersion in the gap modes was found. We suggest that the observed excitations are analogous to magneto-excitons in light rare-earth compounds, but are an intrinsic property of a simple Heisenberg Hamiltonian for the S=1/2 magnetic bilayer.
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