Microscopic description of the surface dipole plasmon in large NaN clusters (950 < N < 12050)

Abstract

Fully microscopic RPA/LDA calculations of the dipole plasmon for very large neutral and charged sodium clusters, NaNZ+, in the size range 950 < N < 12050 are presented for the first time. 60 different sizes are considered altogether, which allows for an in-depth investigation of the asymptotic behavior of both the width and the position of the plasmon.

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