Magnon splitting induced by charge ordering in NaV2O5

Abstract

We consider the effects of charge ordering in NaV2O5 (below TSP) on the exchange constants and on the magnon dispersion. We show that the experimentally observed splitting of the magnon branches along the a direction is induced by charge ordering. We find that one can distinguish between the proposed 'zig-zag' and 'in-line' patterns of charge ordering. Only the zig-zag ordering is consistent with the experimental results regarding (i) the unusual intensity modulation observed in magnetic neutron scattering, (ii) the reduction in the intra-ladder exchange constant below TSP, and (iii) the magnon dispersion along a. We estimate the inter-ladder exchange constant to be 1.01meV=11.7K for T>TSP.

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