Pattern Formation on the Edge of Chaos: CO Oxidation on Pt(110) under Global Delayed Feedback
Matthias Bertram, Michael Pollmann, Harm H. Rotermund, Alexander S. Mikhailov, Gerhard Ertl
Abstract
Experiments with catalytic CO oxidation on Pt(110) show that chemical turbulence in this system can be suppressed by application of appropriate global delayed feedbacks. Different spatiotemporal patterns, seen near a transition from turbulence to uniform oscillations, are investigated. Using a method based on the Hilbert transform, spatial distributions of local phase and amplitude in such patterns are reconstructed from the experimental data. The observed phenomena are reproduced in simulations using a theoretical model of the reaction.
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