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Coherent control of nuclear spin isomers of molecules: The role of molecular motion

P. L. Chapovsky

physics.chem-pharXiv:physics/0109063

Abstract

Molecular center-of-mass motion is taken into account in the theory of coherent control of nuclear spin isomers of molecules. It is shown that infrared radiation resonant to the molecular rovibrational transition can substantially enrich nuclear spin isomers and speed up their conversion rate.

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