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Laser controlled molecular switches and transistors

Jörg Lehmann, Sébastien Camalet, Sigmund Kohler, Peter Hänggi

physics.chem-pharXiv:physics/0205060

Abstract

We investigate the possibility of optical current control through single molecules which are weakly coupled to leads. A master equation approach for the transport through a molecule is combined with a Floquet theory for the time-dependent molecule. This yields an efficient numerical approach to the evaluation of the current through time-dependent nano-structures in the presence of a finite external voltage. We propose tunable optical current switching in two- and three-terminal molecular electronic devices driven by properly adjusted laser fields, i.e. a novel class of molecular transistors.

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