Analytic pulse design for selective population transfer in many-level quantum systems: maximizing amplitude of population oscillations

Abstract

State selective preparation and manipulation of discrete-level quantum systems such as atoms, molecules or quantum dots is a the ultimate tool for many diverse fields such as laser control of chemical reactions, atom optics, high-precision metrology and quantum computing. Rabi oscillations are one of the simplest, yet potentially quite useful mechanisms for achieving such manipulation. Rabi theory establishes that in the two-level systems resonant drive leads to the periodic and complete population oscillations between the two system levels. In this paper an analytic optimization algorithm for producing Rabi-like oscillations in the general discrete many-level quantum systems is presented.