Orienting coupled quantum rotors by ultrashort laser pulses

Abstract

We point out that the non-adiabatic orientation of quantum rotors, produced by ultrashort laser pulses, is remarkably enhanced by introducing dipolar interaction between the rotors. This enhanced orientation of quantum rotors is in contrast with the behavior of classical paired rotors, in which dipolar interactions prevent the orientation of the rotors. We demonstrate also that a specially designed sequence of pulses can most efficiently enhances the orientation of quantum paired rotors.