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Strong extinction of a laser beam by a single molecule

I. Gerhardt, G. Wrigge, P. Bushev, G. Zumofen, R. Pfab, V. Sandoghdar

quant-pharXiv:quant-ph/0604177

Abstract

We present an experiment where a single molecule strongly affects the amplitude and phase of a laser field emerging from a subwavelength aperture. We achieve a visibility of -6% in direct and +10% in cross-polarized detection schemes. Our analysis shows that a close to full extinction should be possible using near-field excitation.

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