Large Exchange Magnetostriction in a Kagome Antiferromagnet at Room Temperature

Abstract

The pursuit of high-performance magnetostrictive materials is crucial for advancing technologies in sensing, actuation, and microelectromechanical systems. Although pronounced magnetostrictive effects have been observed in a few ferromagnets, a systematic exploration of magnetostriction across a broader range of antiferromagnets remains limited. Here, we report the observation of large magnetostriction in the kagome antiferromagnet YMn6Sn6. Under a magnetic field, the system undergoes a field-induced evolution from a helical magnetic ground state toward a collinear field-polarized state, accompanied by a large anisotropic lattice strain and a substantial volume magnetostriction exceeding 400 ppm at room temperature. Remarkably, the magnetostrictive response remains nearly fully reversible up to 9 T with nearly hysteresis-free behavior, effectively minimizing the energy dissipation commonly associated with domain-wall pinning. Combined experimental measurements and theoretical calculations reveal that the large, nearly hysteresis-free magnetostriction originates from the competition between intralayer ferromagnetic and interlayer exchange interactions. This exchange-driven magnetoelastic coupling further gives rise to a strongly direction-dependent lattice distortion pathway. This work establishes kagome helimagnets as a tunable platform for low-dissipation magnetoelastic functionalities and responsive magnetomechanical applications.