Incommensurate lattice distortion in the high temperature tetragonal phase of La2-x(Sr,Ba)xCuO4
Shuichi Wakimoto, Hiroyuki Kimura, Masaki Fujita, Kazuyoshi Yamada, Yukio Noda, Gen Shirane, Genda Gu, Hyunkyung Kim, Robert J. Birgeneau
Abstract
We report incommensurate diffuse (ICD) scattering appearing in the high-temperature-tetragonal (HTT) phase of La2-x(Sr,Ba)xCuO4 with 0.07 ≤ x ≤ 0.20 observed by the neutron diffraction technique. For all compositions, a sharp superlattice peak of the low-temperature-orthorhombic (LTO) structure is replaced by a pair of ICD peaks with the modulation vector parallel to the CuO6 octahedral tilting direction, that is, the diagonal Cu-Cu direction of the CuO2 plane, above the LTO-HTT transition temperature Ts. The temperature dependences of the incommensurability δ for all samples scale approximately as T/Ts, while those of the integrated intensity of the ICD peaks scale as (T-Ts)-1. These observations together with absence of ICD peaks in the non-superconducting x=0.05 sample evince a universal incommensurate lattice instability of hole-doped 214 cuprates in the superconducting regime.
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