Crystallization and phase-separation in non-additive binary hard-sphere mixtures
A. A. Louis, R. Finken, J. P. Hansen
Abstract
We calculate for the first time the full phase-diagram of an asymmetric non-additive hard-sphere mixture. The non-additivity strongly affects the crystallization and the fluid-fluid phase-separation. The global topology of the phase-diagram is controlled by an effective size-ratio yeff, while the fluid-solid coexistence scales with the depth of the effective potential well.
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