Overlapping resonances in the control of intramolecular vibrational redistribution
D. Gerbasi, A. S. Sanz, P. S. Christopher, M. Shapiro, P. Brumer
Abstract
Coherent control of bound state processes via the interfering overlapping resonances scenario [Christopher et al., J. Chem. Phys. 123, 064313 (2006)] is developed to control intramolecular vibrational redistribution (IVR). The approach is applied to the flow of population between bonds in a model of chaotic OCS vibrational dynamics, showing the ability to significantly alter the extent and rate of IVR by varying quantum interference contributions.
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