Study of the intrinsic resolution of LaBr3(Ce,Sr) and NaI(Tl) crystals

Abstract

The Gravitational wave burst high-energy Elec?tromagnetic Counterpart All-sky Monitor (GECAM) utilizes a large number of LaBr3 and NaI(Tl) crystals as sensitive materials for its gamma-ray detectors. To address the fitting issues of the energy resolution curves in the ground calibration of the GECAM detectors, this work conducts a comprehensive testing and comparative study of the energy resolution of 1-inch LaBr3(Ce,Sr) and NaI(Tl) crystals produced from the same batch. We employed a Hard X-ray Calibration Facility (HXCF), a PMT single-photoelectron calibration system, and Geant4 Monte Carlo simulation tools to quantify seven factors influencing energy resolution. The results indicate that the contributions of various components to energy resolution differ, with pho?toelectron statistical fluctuations and intrinsic resolution being predominant. For 100 keV X-rays, the total energy resolution of the LaBr3(Ce,Sr) crystal is 3.71% \pm 0.03% (expressed as 1-σ), with a contribution from photoelectron statistical fluctuations of 2.69% \pm 0.00% and an intrinsic resolution of 2.45% \pm 0.05%. For 100 keV X-rays, the total energy resolution of the NaI(Tl) crystal is 4.41% \pm 0.14% (expressed as 1-σ), with a contribution from photoelectron statistical fluctuations of 3.20% \pm 0.00% and an intrinsic resolution of 2.90% \pm 0.21%. We discussed the sources of intrinsic resolution, and the results indicate that the intrinsic resolution of the LaBr3(Ce,Sr) crystal primarily arises from luminescence non-proportionality, while that of the NaI(Tl) crystal mainly stems from fluctuations during energy transfer. This study emphasizes precise and specific experimental measurements and comparative research, demonstrating that both factors are important contributors to intrinsic resolution.